MBE growth and structural and electrochemical characterization of tin oxide and indium tin oxide nanoparticles grown on silicon for Li-ion battery anodes

Michal J. Osiak, Eileen Armstrong, Tadhg Kennedy, Clivia M.Sotomayor Torres, Kevin M. Ryan, Colm O'Dwyer

Research output: Chapter in Book/Report/Conference proceedingConference contributionpeer-review

2 Citations (Scopus)

Abstract

Tin oxide (SnO2) is considered a very promising material as a high capacity Li-ion battery anode. Typically, the electrochemical performance of tin oxide based anodes is dependent on various factors such as their size and composition. Here, we demonstrate how defined dispersion of nanostructures can improve the understanding of the relationship between the electrode performance and its architecture. Two different types of well-defined hierarchical Sn@SnO2 core-shell nanoparticle dispersions were prepared by molecular beam epitaxy (MBE) on silicon, composed of either amorphous or polycrystalline SnO2 shells. Sn doped In2O3 (ITO) NP dispersions are also demonstrated from MBE nanoparticle growth. Preparation of SnO2 and related materials by highly defined MBE growth as a model system allows a detailed examination of the influence of material dispersion or nanoarchitecture on the performance of active electrode materials.

Original languageEnglish
Title of host publicationNanoarchitectures for Energy Storage
PublisherElectrochemical Society Inc.
Pages1-10
Number of pages10
Edition10
ISBN (Print)9781607684626
DOIs
Publication statusPublished - 2013
Externally publishedYes
EventSymposium on Nanoarchitectures for Energy Storage - 223rd Meeting of the Electrochemical Society - Toronto, ON, Canada
Duration: 12 May 201316 May 2013

Publication series

NameECS Transactions
Number10
Volume53
ISSN (Print)1938-5862
ISSN (Electronic)1938-6737

Conference

ConferenceSymposium on Nanoarchitectures for Energy Storage - 223rd Meeting of the Electrochemical Society
Country/TerritoryCanada
CityToronto, ON
Period12/05/1316/05/13

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